An Experimental Study on the Operating Parameters of Ultrasound-assisted Oxidative Desulfurization
Publish Year: 1398
نوع سند: مقاله ژورنالی
زبان: English
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شناسه ملی سند علمی:
JR_IJOGST-8-3_001
تاریخ نمایه سازی: 6 خرداد 1399
Abstract:
In this research, the effects of important parameters, including the molar ratio of acetic acid to sulfur(S) , sonication time, temperature, and hydrogen the molar ratio of peroxide to sulfur on the performance of ultrasound-assisted oxidative desulfurization were studied using the response surface method (RSM). To this end, a model fuel containing n-decane and dibenzothiophene at a concentration of 1000 ppm was used. It was found out that the temperature and acetic acid/S molar ratio were the most influencing parameters affecting the conversion of sulfur compound. The synergistic effects of the parameters were also investigated, and it was discovered that the maximum conversion of dibenzothiophene reached 98.59% when H2O2/S, acetic acid/S, temperature, and sonication time were set to 167, 330, 80 °C, and 30 min respectively. Finally, the apparent kinetics of dibenzothiophene oxidation and the activation energy of reaction were presented.
Keywords:
Ultrasound-assisted Oxidative Desulfurization (UAOD) , Liquid Hydrocarbon Fuel , Dibenzothiophene , Model Fuel
Authors
Seyede Leila Ebrahimi
Ph.D. Candidate, Gas Engineering Department, Petroleum University of Technology (PUT), Ahwaz, Iran
Mohammadreza Khosravi-Nikou
Associate Professor, Gas Engineering Department, Petroleum University of Technology (PUT), Ahwaz, Iran
Seyed Hassan Hashemabadi
Professor, School of Chemical Engineering, Iran University of Science and Technology, Tehran, Iran
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