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Paper
Title

Bimetallic MOFs as Catalysts for Efficient and Totally Selective Oxidation of Benzylic Alcohols at Ambient Conditions

فصلنامه شیمی معدنی، دوره: 5، شماره: 1
Year: 1400
COI: JR_ICR-5-1_001
Language: EnglishView: 133
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Authors

Alireza Farrokhi - Department of Chemistry, Faculty of Science, University of Birjand, Birjand, ۹۷۱۷۹-۴۱۴ Iran
Maryam Asaadzadeh - Department of Chemistry, Faculty of Science, University of Birjand, Birjand, ۹۷۱۷۹-۴۱۴ Iran
Fahimeh Feizpour - Department of Chemistry, Faculty of Science, University of Birjand, Birjand, ۹۷۱۷۹-۴۱۴ Iran

Abstract:

The catalytic activity of bimetallic MOFs known as STA-۱۲(M۱, M۲)(M۱,۲= Mn, Fe, Co) was investigated in the oxidation of benzylic alcohols to corresponding aldehydes at ambient conditions. The oxidation reaction with Na۲S۲O۴/TBHP (tert-Butyl hydroperoxide) mixture shows total selectivity and excellent efficiency under desired reaction times. The heterogeneous catalyst displays high reusability and stability for the ten consecutive reactions without decreasing in yield and selectivity. To identify radical species responsible for the oxidation process, selective radical scavenging experiments were performed and a purposed oxidation mechanism was discussed.

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This Paper COI Code is JR_ICR-5-1_001. Also You can use the following address to link to this article. This link is permanent and is used as an article registration confirmation in the Civilica reference:

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Farrokhi, Alireza and Asaadzadeh, Maryam and Feizpour, Fahimeh,1400,Bimetallic MOFs as Catalysts for Efficient and Totally Selective Oxidation of Benzylic Alcohols at Ambient Conditions,https://civilica.com/doc/1189522

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