MTO reaction over SAPO-34 catalysts synthesized by different times of crystalization
Publish place: 15th Iranian Natioanl Congress of Chimical Engineering
Publish Year: 1393
نوع سند: مقاله کنفرانسی
زبان: English
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شناسه ملی سند علمی:
ICHEC15_344
تاریخ نمایه سازی: 19 تیر 1394
Abstract:
Effect of crystalization time on the catalytic performance of SAPO-34 catalyst have been investigated in conversion of methanol to light olefins. SAPO-34 catalysts were synthesized by using different crystalization times at 190̊C. The prepared samples were characterized by XRD, SEM and FTIR techniques. The catalytic performance of the synthesized catalysts was tested in MTO reaction at 410°C and WHSV of 6.5 h-1. Time of crystallization were found out as the significant parameter for controlling crystallinity and purity, particle size, morphology and content of hydroxyl groups of the product. all the samples showed cubic morphology and according to the XRD, the sample prepared at 463 K and 24h possessed the best crystallinity with the optimum crystal size. In the methanol conversion to olefins over SAPO-34 catalysts, this sample showed highest yield of light olefins (81.5 %wt) in 100% methanol conversion
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Authors
f Kalantar Kohdami
Department of Chemical Engineering, Tarbiat Modares University, Tehran
j Towfighi Darian
Department of Chemical Engineering, Tarbiat Modares University, Tehran
h Nemati Arbatani
Department of Chemical Engineering, Tarbiat Modares University, Tehran
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